In many regions aerosol-cloud interactions are perturbed by increasing amounts of anthropogenic aerosol particles.
In this respect, changes in cloud albedo, cloud lifetime and the amount of precipitation exert the greatest influence. For Europe knowledge about the emissions and concentrations of air pollutants, and in particular information on aerosols and their precursor gases, is quite comprehensive. In addition, measurements and model calculations indicate the strong variability of this pollution plume owing to changing emissions, chemical transformations, deposition and long-range transport of manifold species, all depending on season and weather type (see e.g. Eliassen and Saltbones, 1983, Krüger and Tuovinen, 1997, EMEP – The European Monitoring and Programme, selleck compound 2004, Schaap et al., 2004, Van Dingenen et al., 2004 and Putaud et al., 2004). During the late 1980s, enormous amounts of particulate matter and aerosol precursor gas emissions, such check details as sulphur dioxide, nitrogen oxides and ammonia, made a strong contribution to the aerosol load over Europe. The extraordinarily
high sulphur dioxide emissions in the former German Democratic Republic (GDR), which amounted to even more than 5 Tg per year, were of major importance to secondary aerosol particle formation. The sizeable contributions from elevated point sources around Halle, Leipzig and Cottbus resulted in pronounced spatial differences of sulphur dioxide (SO2) and particulate matter (PM) concentrations in air. Such an increase in air pollution lead to reduced extinction and altered cloud optics. In Germany Liepert & Kukla (1997) found a statistically significant decrease in the mean annual surface global solar radiation between 1964 and 1990 under completely overcast skies. selleckchem This result can be potentially explained by an increase in cloud optical thickness, changing cloud types, or by human impact on aerosol cloud-mediated processes. The collapse of the Eastern Bloc in 1989 led to significant reductions in industrial activities and thus atmospheric pollution.
A pronounced declining trend was observed in the so-called ‘Black Triangle’; this name refers to the enormous damage to human health and ecosystems caused by soot. This area, covering the southern part of Saxony (Germany), northern Bohemia (Czech Republic) and south-western Lower Silesia (Poland), is a prominent example of the extensive use of lignite deposits in Europe. Stjern et al. (2011) analysed the visibility changes in the ‘Black Triangle’ between 1983 and 2008. They confirmed that the strong reductions in SO2 and PM emissions in central Europe, i.e. a 90% decrease of SO2 emissions and a 72% decrease of measured sulphate concentrations, improved the mean horizontal visibility in the ‘Black Triangle’ from 11 to 27 km between 1983 and 2008.